Feel free to post multiple suggestions for different genres. For example, atmospheric, sci-fi, adventure-like, etc.
Agreed on Persona 5, and I really need to play Persona 4 (it’s on my list but stupid life gets in the way).
Two other picks:
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The original Lunar: The Silver Star on SegaCD. I never played the remakes on other systems but I know they changed significant parts of the soundtrack in those games, while the SegaCD version just hit perfectly for me.
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Final Fantasy Tactics. One of the few soundtrack CDs I imported when those were a thing and could listen to and instantly recall fond memories of playing the game.